Well, often a dumped litter box and a mess is their non-verbal way of communicating that they are unhappy about something. Probably related to the litter pan or housing.
I’m thinking she may feel that her dog crate home is too confining, and wants out. Have you considered getting her an X-pen that you could set up that would give her more space to roam and get comfortable in? If you go above and look at the habitat section under Bunny Info on the green banner, you’ll see some very creative housing. You don’t need to build anything too elaborate, but my guess is a big bunny wants a lot more space.
That said, a bunny may also toss litter if she doesn’t like that type or brand. Did you ever change her litter? My bunny surprised my by tossing the soft type and preferring the pellet type. I knew this, after spending on sample bags, because she stopped the tossing once she was pleased.
Finally, you can buy a litter pan that comes with a screw mechanism attached, which I use, that goes outside the bars and hooks onto the pan so it stays put. It’s a corner pan. I got it at a petshop. Also, if you just want a plain litter pan, poke a hole into the side of it, not far from the top, sand down the rough edges of the hole for safety, and run a tie through it. Hook the tie around the outside of the cage bar to hold it in place and to make it available for you to untie when it’s time to clean.
Some folks use dog clips, but I don’t exactly know how to clip a litter pan with one. It may be easier than a hole and tie if you can find one that fits.